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After signing with Epic Records, Moore began working on her debut album.
While recording the album, Moore had to leave Bishop Moore Catholic High School when she was only in the ninth-grade, but continued receiving her education from tutors.
Allmusic called the album a "leap to musical maturity," This made it Moore's highest debut on the chart, and highest-peaking album to date, but it is her lowest-selling, and her first album not to be certified by the RIAA.
Moore's cover of XTC's 1982 song "Senses Working Overtime" was released as the album's second single and also failed to have any chart success.
Moore also voiced Princess Rapunzel in the Disney animated fantasy musical comedy film Tangled (2010), the short film Tangled Ever After (2012), and the Disney Channel television series Tangled: The Series (2017–present).
It received generally mixed reviews from critics when it was released, and Moore continued to be compared to other teen pop singers.I Wanna Be with You was released as Moore's debut album in a number of countries.The album received generally mixed reviews and criticism because it was a remix album and not a true follow-up.Moore's cover of Carole King's 1971 song "I Feel the Earth Move" was also on the compilation album Love Rocks from LGBT rights supporters.Moore's second compilation album, Candy, was released on April 5, 2005.